Tuning Overbias Plasmon Energy and Intensity in Molecular Plasmonic Tunneling Junctions by Atomic Polarizability.

Wei Du, Xiaoping Chen, Tao Wang, Qianqi Lin, Christian A Nijhuis

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Article in Journal of the American Chemical Society, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

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2 · The registry

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5 · Who and what money

Authors and funding

5 authors.

Wei DuDepartment of Chemistry, National University of Singapore, 3 Science Drive 3, 117543 Singapore, Singapore.ORCID 0000-0001-8678-8844

Xiaoping ChenDepartment of Chemistry, National University of Singapore, 3 Science Drive 3, 117543 Singapore, Singapore.

Tao WangDepartment of Chemistry, National University of Singapore, 3 Science Drive 3, 117543 Singapore, Singapore.ORCID 0000-0003-2250-7569

Qianqi LinHybrid Materials for Optoelectronics Group, Department of Molecules and Materials, MESA+ Institute for Nanotechnology, Molecules Center and Center for Brain-Inspired Nano Systems, Faculty of Science and Technology, University of Twente, 7500AE Enschede, The Netherlands.ORCID 0000-0001-7578-838X

Christian A NijhuisHybrid Materials for Optoelectronics Group, Department of Molecules and Materials, MESA+ Institute for Nanotechnology, Molecules Center and Center for Brain-Inspired Nano Systems, Faculty of Science and Technology, University of Twente, 7500AE Enschede, The Netherlands.ORCID 0000-0003-3435-4600

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Plasmon excitation in molecular tunnel junctions is interesting because the plasmonic properties of the device can be, in principle, controlled by varying the chemical structure of the molecules. The plasmon energy of the excited plasmons usually follows the quantum cutoff law, but frequently overbias plasmon energy has been observed, which can be explained by quantum shot noise, multielectron processes, or hot carrier models. So far, clear correlations between molecular structure and the plasmon energy have not been reported. Here, we introduce halogenated molecules (HS(CH

Identifiers

PMID38940772

DOI10.1021/jacs.4c05544

PMCPMC11311224

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