ArticleScience advances2024
Observation of dynamic nuclear polarization echoes.
Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
What it found
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Who cites it
4 citing papers in PubMed.
- Symmetry-based pulsed DNP and EPR sequences.Science advances · 2026Article
- Optimal control of spin systems.Science advances · 2026Review
- In situ learning-based spin engineering of pulsed dynamic nuclear polarization.Science advances · 2026Article
- Coherent Control over Nuclear Hyperpolarization Using an Optically Initializable Chromophore-Radical System.Journal of the American Chemical Society · 2025Article
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
It is demonstrated that the time evolution of the electron-nuclear polarization transfer process during pulsed dynamic nuclear polarization (DNP) can be reversed on a microsecond timescale, leading to the observation of DNP echoes. The DNP echoes are induced by consecutive application of two pulse trains that produce effective Hamiltonians that differ only in the sign of the effective hyperfine coupling. The experiments have been performed on a frozen solution of trityl radicals in water/glycerol on a homebuilt X-band electron paramagnetic resonance/DNP spectrometer at 80 kelvins. We envisage that DNP echoes will play an important role in future development of pulsed DNP for sensitivity-enhanced nuclear magnetic resonance, hyperfine spectroscopy, and quantum sensing.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the Socratic graph.