Evidence mapPaperPMID 40013616Full record

ArticleAngewandte Chemie (International ed. in English)2025

Site-Selective C─H Bond Functionalization of Sugars.

Elena V Stepanova, Andrey Shatskiy, Ivan Doroshenko, Peter Dinér, Markus D Kärkäs

Abstract read
In one paragraph

Article in Angewandte Chemie (International ed. in English), 2025. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.

0numbers the graph read from it
0cells of the map it votes in
4citing papers in PubMed
field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

4 citing papers in PubMed.

  1. Review
  2. Site-Selective Distal Arylation of Sugars Enabled by Cyclic Acetals.Journal of the American Chemical Society · 2026
    Article
  3. Review
  4. Site-Selective C─H Bond Functionalization of Sugars.Angewandte Chemie (International ed. in English) · 2025
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Elena V StepanovaDepartment of Chemistry, KTH Royal Institute of Technology, Teknikringen 30, Stockholm, SE-100 44, Sweden.
Andrey ShatskiyDepartment of Chemistry, KTH Royal Institute of Technology, Teknikringen 30, Stockholm, SE-100 44, Sweden.
Ivan DoroshenkoDepartment of Chemistry, KTH Royal Institute of Technology, Teknikringen 30, Stockholm, SE-100 44, Sweden.
Peter DinérDepartment of Chemistry, KTH Royal Institute of Technology, Teknikringen 30, Stockholm, SE-100 44, Sweden.
Markus D KärkäsDepartment of Chemistry, KTH Royal Institute of Technology, Teknikringen 30, Stockholm, SE-100 44, Sweden.

Funding

Magnus Bergvall Foundation, Ministry of Education and Science of the Russian Federation 075-03-2024-118/1Olle Engkvist Foundation, Swedish Research Council 2020-04764Olle Engkvist Foundation, Swedish Research Council 2023-04482Olle Engkvist Foundation, Swedish Research Council 2024-04263the Swedish Research Council 2022-06725
6 · The paper itself

Abstract

Non-typical C-functionalized sugars represent a prominent yet hardly accessible class of biologically-active compounds. The available synthetic methodologies toward such sugar derivatives suffer either from an extensive use of protecting groups, requiring long and laborious synthetic manipulations, or from limited predictability and noncontrollable site-selectivity of the employed C-functionalization reactions. In this work, we disclose an alternative synthetic methodology toward nontypical sugars that allows facile, site-selective, and stereocontrolled C-functionalization of sugars through a traceless tethering approach. The described silyl-based redox-active tethering group appends directly to the unprotected sugar substrate and mediates the C-functionalization reaction through a photochemically-promoted 1,6-hydrogen atom transfer (HAT) mechanism, while transforming into a readily-removable silyl protecting group. The protocol is compatible with a variety of unprotected carbohydrate substrates featuring sensitive aglycons and a diverse set of coupling partners, providing a straightforward and scalable route to pharmaceutically relevant C-functionalized carbohydrate conjugates.

Indexed as

CarbohydratesCarbonHydrogenSugarsMolecular StructureOxidation-ReductionCarbohydratesCarbonHydrogenSugarsCarbohydratesC─H bond activationPhotoredox catalysisRadicalsVisible light

Identifiers

PMID40013616
PMCPMC12051779

What Socratic holds

Textmetadata
LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the Socratic graph.