ArticleAngewandte Chemie (International ed. in English)2026
Water-Splitting-Suppressed High-Capacity Bipolar Electrodes Enabled by Topochemical Electron Buffering for Symmetric Aqueous Batteries.
Article in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Symmetric aqueous batteries (SABs) that employ bipolar materials as electrodes have attracted tremendous attention due to their intrinsic safety and satisfactory capacity, while they still suffer from water-splitting and thus a narrow voltage window. In this work, we propose a novel topochemical design of introducing an electron buffer (EB) to control the electron stream when working, which efficiently attenuates the electron flow toward the water-splitting reactions at the voltage ends. Careful measurements confirm the sharp reduction of current density applied for water-splitting due to the EB effect. Theoretical calculations for voltage end verify the lower surface electron density of EB-involved electrode than that of EB-excluded electrode, demonstrating the superiority of this EB design in suppressing charge shock for water splitting. Consequently, the charging/discharging plateau of the assembled SABs based on EB increases ∼0.16 V, as well as a high capacity of 80.7 mA h g
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