ArticleNPJ climate and atmospheric science2026
High-resolution aerosol liquid water content in the contiguous United States using machine learning.
Article in NPJ climate and atmospheric science, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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13 authors.
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Abstract
Aerosol liquid water content (ALWC) plays an important role in climate and public health by influencing aerosol formation, chemical composition, and toxicity. However, ALWC remains sparsely measured and poorly constrained across space and time, despite its large variability. In this study, we derived a high-resolution (1 km × 1 km, daily) ALWC dataset for the contiguous US from 2000 to 2019. The dataset was generated by training machine learning (ML) models on outputs from a chemical transport model (GEOS-Chem) to capture the thermodynamic relationships between ALWC and relevant predictors, then applying these relationships to high-resolution, biased-corrected input datasets. Compared with GEOS-Chem simulations, the ML-based dataset better captures daily variations and spatial heterogeneity in ALWC. The predicted ALWC levels are highest in the Midwest US and lowest in the Western US, largely driven by regional differences in PM
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