ReviewAngewandte Chemie (International ed. in English)2026
Water, Alcohols, Amines, and Amides as Formal Hydrogen-Atom-Transfer Reagents Through Activation With Redox-Active Lewis Acids.
Review in Angewandte Chemie (International ed. in English), 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
The O─H and N─H bonds of protic molecules such as water, alcohols, amines, or amides typically resist hydrogen-atom abstraction because of the high energy of the resulting heteroatom-centered radical intermediates. However, association of the protic molecules with redox-active Lewis acids provides stabilization of the generated reactive radical intermediates and enables the ligated protic molecules to serve as hydrogen-atom donors or proton-coupled-electron-transfer reagents. This review presents an overview of applications of this bond-weakening principle in organic synthesis and attempts to illustrate the breadth of systems that enable such reactivity.
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