ArticleFaraday discussions2026
Electrolyte and gas flow rate balance in flow cells for lithium-mediated ammonia electrosynthesis.
Article in Faraday discussions, 2026. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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5 authors.
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Abstract
The electrochemical lithium-mediated nitrogen reduction reaction (Li-NRR) has emerged as a leading approach for ammonia electrosynthesis under mild conditions, particularly in continuous flow-cell configurations. Despite the rapid progress of this strategy, as well as the remarkable efforts in electrolyte composition engineering and solid-electrolyte-interphase layer understanding, the impact of architecture-level parameters remains unclear and is often entangled with the intrinsic process reactivity and selectivity. Here, we systematically investigate the influence of electrolyte and nitrogen-gas flow rates on Li-NRR performance in a flow cell, attempting to decouple the effect of device-level parameters from reaction chemistry in determining activity, selectivity, and stability of the system. By balancing liquid and gas flows, we demonstrate stable device operation even at high electrolyte flow rates (18 mL min
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